Vinylcyclopropanecarboxylates having an excellent insecticidal activity and a property harmless to mammals and cattle, of the formula, ##SPC1## Wherein R is 2-propargyl-3-methyl-2-cyclopentene-1-one- ##SPC2## Wherein R.sub.1 is allyl, propargyl, benzyl, thenyl, furylmethyl or phenoxy, R.sub.2 is hydrogen, or R.sub.1 and R.sub.2 are bonded at respective ends to form a polymethylene group having 3 to 4 carbon atoms, and X is oxygen or sulfur.